Plasmonic quasicrystals for designable ultra broadband transmission enhancement and second harmonic generation

Quasi-crystals are intriguing as they exhibit rotational symmetry and long range ordering but lack translational symmetry. 2-dimensional metal-dielectric patterns are interesting to make use of surface plasmon polariton (SPP) mediated local field enhancement and for near dispersionless SPP modes. In plasmonic crystals, the orientation and periodicity of the pattern dictate the polarization response and the discrete plasmon resonances while the interfaces define the plasmon dispersion. However, unique properties of plasmonic quasicrystals lead to polarization independence, designable k-space and broadband transmission enhancement due to SPP mediation. These are useful in many applications like energy harvesting, nonlinear optics and quantum plasmonics. We demonstrate design and fabrication of large area quasicrystal air hole patterns of pi/5 symmetry in metal film in which broadband, launch angle and polarization independent transmission enhancement as well as broadband second harmonic generation are observed. Designable transmission response, other symmetries and tilings are possible.