Optical clocks based on linear ion chains with high stability and accuracy

2017 
Trapped-ion optical clocks are capable of achieving systematic fractional frequency uncertainties of $10^{-18}$ and possibly below. However, the stability of current ion clocks is fundamentally limited by the weak signal of single-ion interrogation. We present an operational, versatile platform for extending clock spectroscopy to arrays of Coulomb crystals consisting of several tens of ions, while allowing systematic shifts as low as $10^{-19}$. The concept is applicable to all clock transitions with low differential electric quadrupole moments. We observe 3D excess micromotion amplitudes of all individual ions inside a Coulomb crystal with nm resolution and prove that the related frequency shifts can be controlled simultaneously at the $10^{-19}$ level. Using this method, we demonstrate regions of $400$ $\mu$m and $2$ mm length in our trap array with time dilation shifts due to micromotion close to $1\times10^{-19}$ and below $10^{-18}$, respectively. Further measurements of the trapping environment and cooling dynamics calculations for mixed In${}^+$ / Yb${}^+$ crystals show that achievable clock uncertainties due to multi-ion operation in our setup are below $1\times10^{-19}$. This work will enable clock operation with multiple ions and open up the possibility of new interrogation schemes which allow optical clock stabilities beyond classical limits.
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