Abnormal dependence of strong-field-ionization-induced nitrogen lasing on polarization ellipticity of the driving field
2013
We experimentally investigate lasing behaviors of population-inverted N${}_{2}$ ions for the transitions between the vibrational level ($v$\ensuremath{'} = 0) of excited electronic $B$ \ensuremath{\Sigma}${}_{u}$${}^{+}$ state and the two lowest vibrational levels ($v$ = 0, 1) of the ground $X$ \ensuremath{\Sigma}${}_{g}$${}^{+}$ state in an elliptically polarized laser field. It is found that, as the polarization of the pump laser evolves from linear to circular, the lasing signal for the 0 \ensuremath{\rightarrow} 0 transition at 391 nm first increases with a maximum enhancement of \ensuremath{\sim}40% at the ellipticity of 0.3 and then decreases, whereas for the 0 \ensuremath{\rightarrow} 1 transition at 428 nm, the lasing signal decreases monotonically. This difference between the 391- and 428-nm lasing signals is ascribed to the high sensitivity of the strong-field response of the molecular ion to molecular vibrations, which indicates the possibility to control the vibrational state distribution of molecules by tuning the ellipticity of the laser pulse.
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