Origin of magnetic anisotropy in the spin ladder compound (C$_5$H$_{12}$N)$_2$CuBr$_4$.
2019
The $S=1/2$ spin ladder compound (C$_5$H$_{12}$N)$_2$CuBr$_4$ (BPCB) is studied by means of high-resolution inelastic neutron scattering. In agreement with previous studies we find a band of triplet excitations with a spin gap of $\sim0.8$~meV and a bandwidth of $\sim0.6$~meV. In addition, we observe a distinct splitting of the triplet band of $50(1)$~$\mu$eV or $40(2)$~$\mu$eV at the band minimum or maximum, respectively. By comparison to a strong coupling expansion calculation of the triplet dispersion for a spin ladder with anisotropic exchange, weakly anisotropic leg interactions are identified as the dominant source of magnetic anisotropy in BPCB. Based on these results, we discuss the nature of magnetic exchange anisotropy in BPCB and in related transition-metal insulators.
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