A flat band at the chemical potential of a Fe1.03Te0.94S0.06 superconductor observed by angle-resolved photoemission spectroscopy

The electronic structure of superconducting Fe1:03Te0:94S0:06 has been studied by angle-resolved photoemission spectroscopy (ARPES). Experimental band topography is compared to the calculations using the methods of Korringa‐Kohn‐Rostoker (KKR) with the coherent potential approximation (CPA) and the linearized augmented plane wave with local orbitals (LAPWC LO) method. The region of the0 point exhibits two hole pockets and a quasiparticle peak close to the chemical potential ( ) with undetectable dispersion. This flat band with mainly d z 2 orbital character is most likely formed by the top of the outer hole pocket or is evidence of a third hole band. It may cover up to 3% of the Brillouin zone volume and should give rise to a Van Hove singularity. Studies performed for various photon energies indicate that at least one of the hole pockets has a two-dimensional character. The apparently nondispersing peak at is clearly visible for 40 eV and higher photon energies, due to an effect of the photoionization cross-section rather than band dimensionality. Orbital characters calculated by LAPWC LO for stoichiometric FeTe do not reveal the flat dz2 band but are in agreement with the experiment for the other dispersions around0 in Fe1:03Te0:94S0:06. (Some figures may appear in colour only in the online journal)