Development of a low-level 39Ar calibration standard – Analysis by absolute gas counting measurements augmented with simulation

Abstract This paper describes the generation of 39 Ar, via reactor irradiation of potassium carbonate, followed by quantitative analysis (length-compensated proportional counting) to yield two calibration standards that are respectively 50 and 3 times atmospheric background levels. Measurements were performed in Pacific Northwest National Laboratory's shallow underground counting laboratory studying the effect of gas density on beta-transport; these results are compared with simulation. The total expanded uncertainty of the specific activity for the ~50× 39 Ar in P10 standard is 3.6% (k=2).