Unusual spin dynamics in the low-temperature magnetically ordered state of Ag$_{3}$LiIr$_{2}$O$_{6}$

2021 
Recently, there have been contrary claims of Kitaev spin-liquid behaviour and ordered behavior in the honeycomb compound Ag$_3$LiIr$_2$O$_6$ based on various experimental signatures. Our investigations on this system reveal a low-temperature ordered state with persistent dynamics down to the lowest temperatures. This is confirmed by clear oscillations in the muon spin relaxation ($\mu$SR) time spectrum below 9 K till 52 mK. Coincidentally in $^7$Li nuclear magnetic resonance, a wipe-out of the signal is observed below $\sim$10 K strongly indicating magnetic order. This is supported by our density functional theory calculations which show significant Heisenberg terms in the spin Hamiltonian that favor magnetic ordering. The $^7$Li shift and spin-lattice relaxation rate also show anomalies at $\sim$50 K. They are likely related to the onset of dynamic magnetic correlations, but their origin is not completely clear. Detailed analysis of our $\mu$SR data is consistent with a co-existence of incommensurate N\'eel and striped environments. A significant dynamical relaxation rate in the ordered phase as seen in $\mu$SR indicates enhanced quantum fluctuations in the ordered state.
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