Quantum metal state and quantum phase transitions in type-II Ising superconducting films.

Recent emergence of two-dimensional (2D) crystalline superconductors has provided a promising platform to investigate novel quantum physics and potential applications. To reveal essential quantum phenomena therein, ultralow temperature transport investigation on high quality ultrathin 2D superconducting films is critically required, although it has been quite challenging experimentally. Here we report a systematic transport study on the macro-size ambient-stable ultrathin PdTe2 films grown by molecular beam epitaxy. Interestingly, a new type of Ising superconductivity in 2D centrosymmetric materials is revealed by the detection of large in-plane critical field more than 6 times Pauli limit. Remarkably, in perpendicular magnetic field, the film undergoes the quantum phase transition from a quantum metal to weakly localized metal with the presence of intermediate quantum Griffiths singularity. Our findings lead to a global phase diagram of two-dimensional superconducting system with strong spin-orbit coupling.