Identification of anthropogenic radionuclides in the Song Hong (Red) and Song Da (Black) river basins of Vietnam

The concentration and distribution of U were measured in zircon samples separated from the streambed sediments collected at different sites along the rivers of northern Vietnam using semiconductor alpha spectrometry and alpha- and fission-track autoradiography. Based on the absolute U content and distribution, we distinguished two groups of zircon grains of different origin. Group 1 zircons have relatively low and uniform U contents ranging from 280 to 440 μg/g. Group 2 zircons are characterized by heterogeneous U distribution and U contents ranging from 490 to 2040μg/g. The determination of absolute alpha activity values and alpha spectrometric characteristics for a number of group 2 zircon grains indicated the presence of relatively short-lived alpha-emitters. These radionuclides are probably 210Po, 232U, 236Pu, 241Am, and 243Am, and all of them can originate exclusively from anthropogenic sources. A comparison of the observed alpha activity values for group 2 zircons with those of group 1 zircons and zircons separated from the suspended colloids in river water samples provided conclusive evidence for traces of anthropogenic radioactive contamination in the Lao Cai, Yen Bai, Tuyen Quang, Thac Ba, Viet Tri, and Hanoi streams flowing in the Song Hong (Red) and Song Da (Black) river basins of northern Vietnam and sourced in the southern regions of the neighboring state.