Pulsed plasma generator development and low-temperature plasma-assisted combustion at atmospheric pressure

This thesis presents an experimental study of the engineering and physics of high-voltage nanosecond-pulsed diffuse discharges, and their application to the enhancement of lean-premixed combustion at atmospheric pressure. The technology development in this work is focused on providing appropriate low-temperature radical pools, and the experiments are aimed at demonstrating the effect of these pools for combustion actuation. The experimental results are focused on the explanation of the physical processes associated with these discharges. The discharge propagation and emission spectrum were examined, the distribution functions of particles along internal energy levels were calculated, and the resulting enhancement of combustion was observed. This work shows that the plasma emission from fuel-lean mixtures is primarily composed of high vibrational populations of electronically excited nitrogen molecules, upon which a low-temperature is measured on the rotational manifold. Previous work shows that these low-temperature excited particles will collide with molecular oxygen, or fuel molecules, to produce species (atomic/molecular ground/excited oxygen, fragmented fuel molecules…) that accelerate chain-branching reactions in the combustion reaction mechanism. This work shows that the majority of the electronically excited vibrational states of nitrogen molecules, in a diffuse discharge, decay rapidly after the application of a high-voltage pulse. These findings set the framework for the implementation of diffuse plasma to laboratory-scale combustion enhancement. As an integral part of this work, the design and development of electrical generators that can produce such a reactive medium in large volume is included, and extensively detailed. An inexpensive solid-state pulse generator, based on commercially available amorphous ferromagnetic materials, is designed and developed to drive capacitive loads. The generator is used to produce large volumes of diffuse plasma and increase the blow off velocity of stagnation flames. To further investigate this enhancement, an optically accessible plasma burner is implemented and used for the detailed study of stagnation flame plasma actuation. This work shows that significant actuation can be provided to a flame, when diffuse plasma is placed upstream, and directly in contact with the combustion front. The displacement of the leading edge of a flame, into the fresh unburned mixture, is measured following a high-voltage actuating pulse. The displacement of the leading edge strongly points toward low-temperature reactivity enhancement. The optical and electrical characteristics of the diffuse plasma are reported for both the non-combusting and combusting flows. These provide a more accurate picture of the thermal characteristics and complex phenomena occurring in this transient discharge. Streamer propagation dynamics and coupled energy measurements are reported to provide further insight regarding the delicate balance that exists between plasma and flame sheet in this experimental…