Phase-Sensitive Sum-Frequency Vibrational Spectroscopy and Its Application to Studies of Interfacial Alkyl Chains
2007
The first general phase-sensitive sum-frequency vibrational spectroscopy (SFVS) was described, which recovers the phase information lost in conventional SFVS measurements. Using a self-assembled monolayer, we demonstrated that this novel technique measures the absolute orientation of surface molecular moieties and is very powerful in resolving spectral features.
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