Ultrathin and Stretchable Rechargeable Devices with Organic Polymer Nanosheets Conformable to Skin Surface

: Ultrathin flexible electronic devices have been attracting substantial attention for biomonitoring, display, wireless communication, and many other ubiquitous applications. In this article, organic robust redox-active polymer/carbon nanotube hybrid nanosheets with thickness of just 100 nm are reported as power sources for ultrathin devices conformable to skin. Regardless of the extreme thinness of the electrodes, a moderately large current density of 0.4 mA cm-2 is achieved due to the high output of the polymers (>10 A g-1 ). For the first time, the use of mechanically robust yet intrinsically soft electrodes and polymer nanosheet sealing leads to the fabrication of rechargeable devices with only 1-µm thickness and even with stretchable properties.