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Molecular beams of elements constituting a crystal and ion beams prepared by ionizing dopant atoms and/or dopant molecules are simultaneously and uniformly directed to a surface of a substrate and a region of the surface which is not required to be doped is simultaneously irradiated with electron beams. The ion beams directed to the regions not to be doped are coupled with the electron beam prior to and on arrival at the region and electrically neutralized. Thus, the crystal grows in some regions without the dopant and the crystal also grows in other regions with the dopant.