Mapping chemical bonding of reaction intermediates with femtosecond X-ray laser spectroscopy

Ph. Wernet,M. Beye,F. M. F. de Groot,S. Düsterer,Kelly J. Gaffney,S. Grübel,Robert W. Hartsock,Franz Hennies,Ida Josefsson,Brian K. Kennedy,Kristjan Kunnus,T. Leitner,T. Mazza,M. Meyer,Dennis Nordlund,Michael Odelius,Wilson Quevedo,P. Radcliffe,Ivan Rajkovic,B. Schlotter,Mirko Scholz,Simon Schreck,Edlira Suljoti,Simone Techert,J. J. Turner,Christian Weniger,Wenkai Zhang,A. Föhlisch

Mapping chemical bonding of reaction intermediates with femtosecond X-ray laser spectroscopy

2013

We determine the pathways in the photo-dissociation reactions of Fe(CO)5 both in the gas phase and in solution by mapping the valence electronic structure of the reaction intermediates with femtosecond X-ray laser spectroscopy.

Keywords:

Spectroscopy
Reaction intermediate
Chemical bond
Femtosecond
Valence (chemistry)
Molecular physics
Electronic structure
X-ray laser
Chemistry
gas phase
Chemical physics
Photochemistry

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