Low-threshold upconverted single-mode lasing from CdS hexagonal microcavities.

Upconversion micro/nanolasers are promising in fundamental physics research and practical applications. However, due to the limitation of gain medium and cavity quality, such lasers still suffer from a high lasing threshold (P th). Herein, upconverted whispering-gallery-mode lasing by two-photon absorption is achieved from CdS microplatelets with single-mode emission and low threshold (∼1.2 mJ cm-2). The threshold is three times lower than the best reported value in previous CdS upconversion lasers. Moreover, wavelength-tunable upconverted single-mode lasing is demonstrated from 510.4 to 518.9 nm with narrow linewidths around 0.85 nm, which is further verified through numerical simulations. In addition, the size-dependent lasing behavior is realized from single-mode to multimode oscillation; the corresponding lasing threshold decreases with increasing cavity edge length (L), following a P th ∝ 1/L 2 relationship. These results underscore the promise of CdS microplatelets for developing chip-level frequency upconversion lasers.