Properties of correlated fission fragments from neutron induced fission of Np-237 at incident neutron energies between 200 keV and 100 MeV

2021 
Data from the neutron-induced fission of major actinides are vital to applications such as nuclear energy, nuclear forensics, nonproliferation and stockpile stewardship. Of particular interest are the average total kinetic energy ($\langle TKE\rangle$) of fission fragments and mass yield distributions. Neptunium-237 is produced in significant quantities in the nuclear fuel cycle. Its presence in spent reactor fuel and $\sim2\times10^6$ year half life make a complete and precise understanding of its production and destruction desirable to inform reactor design. Little $\langle TKE\rangle$ data exist for $^{237}$Np$(n,f)$. This study measured post-neutron emission mass yields and $\langle TKE\rangle$ of correlated fission products from $^{237}$Np$(n,f)$ over a wide range of incident neutron energies. These measurements were made with a twin Frisch-gridded ionization chamber and a thin-backed $^{237}$Np target at the Los Alamos Neutron Science Center - Weapons Neutron Research facility, which provides a collimated beam of neutrons with energies ranging from 100's of keV to 100's of MeV. The data were analyzed using the double-energy method. Pre- and post-neutron emission $\langle TKE\rangle$ values are reported for 54 incident neutron energies in the range $0.20\le E_n \le100.0$ MeV and compared to existing data and models. Pre- and post-neutron emission mass yields are extracted with a resolution of $\sim4$u FWHM and compared to existing data and evaluations. The present data agree with previous results and also with statistical models. A flattening of the $\langle TKE\rangle$ is observed (relative to model predictions) above $E_n = 20.0$ MeV. The interpretation of this discrepancy is unclear as the analysis method's neglect of incomplete momentum transfer as well as pre-equilibrium pre-fission phenomena likely significantly impact the measurement at such high incident neutron energies.
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