Measurements of Neutron Spallation Cross Sections of 12C and 209Bi in the 20- to 150-MeV Energy Range

The neutron spallation cross sections of {sup 12}C and {sup 209}Bi have been measured in the quasimonoenergetic p-{sup 7}Li neutron fields in the 20- and 150-MeV energy range. The irradiation experiments were performed at four cyclotron facilities: (a) the Institute for Nuclear Study (INS), University of Tokyo; (b) the Cyclotron and Radioisotope Center, Tohoku University; (c) the Takasaki Research Establishment (TIARA), Japan Atomic Energy Research Institute; and (d) the Institute of Physical and Chemical Research (RIKEN). The neutron spectrum has been measured with the time-of-flight method using an organic liquid scintillator, and the absolute value of peak neutron fluence has been estimated from the activation method of lithium target at INS, RIKEN, and the proton recoil counter telescope at TIARA. The cross-section data of {sup 12}C(n,2n){sup 11}C and {sup 209}Bi(n,xn) (x = 3.12) reactions are reported. The experimental data were compared with other experimental data [only for {sup 12}C(n2n){sup 11}C and {sup 209}Bi(n,3n){sup 207}Bi reactions] and the ENDF/B-VI high-energy file data. The comparison showed good agreement between the authors data and others. Their data of {sup 209}Bi(n,xn) reactions above 20 MeV and of {sup 12}C(n,2n){sup 11}C reactions above 40 MeV are the first experimental data and will be applied tomore » high-energy neutron spectrometry for the Bi spallation detector.« less