Variability of North Atlantic CO 2 fluxes for the 2000–2017 period estimated from atmospheric inverse analyses
2021
Abstract. We present new estimates of the regional North Atlantic
(15–80 ∘ N) CO 2 flux for the 2000–2017 period
using atmospheric CO 2 measurements from the NOAA long-term surface site
network in combination with an atmospheric carbon cycle data assimilation
system (GEOS-Chem–LETKF, Local Ensemble Transform Kalman Filter). We assess the sensitivity of flux estimates to
alternative ocean CO 2 prior flux distributions and to the
specification of uncertainties associated with ocean fluxes. We present a
new scheme to characterize uncertainty in ocean prior fluxes, derived from a
set of eight surface p CO 2 -based ocean flux products, and which
reflects uncertainties associated with measurement density and
p CO 2 -interpolation methods. This scheme provides improved model
performance in comparison to fixed prior uncertainty schemes, based on
metrics of model–observation differences at the network of surface sites.
Long-term average posterior flux estimates for the 2000–2017
period from our GEOS-Chem–LETKF analyses are − 0.255 ± 0.037 PgC yr −1 for the subtropical basin (15–50 ∘ N) and
− 0.203 ± 0.037 PgC yr −1 for the subpolar region (50–80 ∘ N, eastern boundary at 20 ∘ E). Our basin-scale
estimates of interannual variability (IAV) are 0.036 ± 0.006 and 0.034 ± 0.009 PgC yr −1 for subtropical and subpolar
regions, respectively. We find statistically significant trends in carbon
uptake for the subtropical and subpolar North Atlantic of − 0.064 ± 0.007 and − 0.063 ± 0.008 PgC yr −1 decade −1 ; these trends are
of comparable magnitude to estimates from surface ocean p CO 2 -based
flux products, but they are larger, by a factor of 3–4, than trends estimated from
global ocean biogeochemistry models.
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