Annealing induced coherent evolutions of biaxial strain and antiferromagnetic-insulator phase in La0.625Ca0.375MnO3 films

La0.625Ca0.375MnO3 (LCMO) films with thicknesses between 7 and 54 nm were epitaxially grown on (LaAlO3)0.3(Sr2AlTaO6)0.35 (001) [LSAT (001)] substrates by using pulsed laser deposition. For this epitaxial system, antiferromagnetic-insulator (AFI) state can be controlled by changing the film thickness and annealing time with various epitaxial strain states, although this phenomenon is absent in the relatively thick films or bulk samples. The consistency between magnetization and resistivity data suggests all these interesting transport behaviors are attributed to the fluctuation of AFI volume fractions and their instability. Especially, there are huge low-field magnetoresistance over −54% (32 nm) at 0.1 T and enhanced magnetoresistance over a broad temperature range. Based on these above results, annealing induced coherent evolutions of biaxial strain and AFI phase in LCMO epitaxial films is a consequence of the strain-driven orbital ordered state, and this may make an approach for a possible application o...