Three-dimensional recoil-ion momentum analyses in 8.7 MeV O7+-He collisions

1995 
Using high-resolution recoil-ion momentum spectroscopy we have measured the differential cross sections of single-electron capture and target single-ionization processes for 8.7 MeV O7+-He collisions as functions of scattering angle. A transverse momentum resolution of +or-0.2 au, which corresponds to an angular resolution of about +or-1.5*10-6 rad for the projectile scattering angle, was obtained by intersecting a well collimated O7+ beam with a target of a supersonic He jet from a pre-cooled gas and by measuring the recoil-ion transverse momentum. For the single capture reaction, information on the n-value of the electron final state in O6+ (1snl) is obtained from the longitudinal momentum of the recoil ions. In pure single-electron capture, the dominant contributions to capture were found to be those from the n=4 and higher states, whereas single capture accompanied by the ionization of the second target electron mainly populates n=2 to n=4 states. Furthermore, the measured transverse momentum distribution differs significantly between pure single capture and capture with simultaneous ionization. The measured data for the pure capture process compare favourably with theoretical results based on a molecular-state expansion method. Other experimental data are discussed in terms of the classical overbarrier model.
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