Multi-step shot noise spectrum induced by a local large spin

We use non-equilibrium Green’s function method to analyze the shot noise spectrum of artificial single molecular magnets(ASMM) model in the strong spin–orbit coupling limit in sequential tunneling regime, mainly focusing on the effects of local large spin. In the linear response regime, the shot noise shows 2S + 1 peaks and is strongly spin-dependent.In the nonlinear response regime, one can observe 2S + 1 steps in shot noise and Fano factor. In these steps one can see the significant enhancement effect due to the spin-dependent multi-channel process of local large spin, which reduces electron correlations.