Theoretical study of scattering in graphene ribbons in the presence of structural and atomistic edge roughness

2019 
We investigate the diffusive electron-transport properties of graphene ribbons and nanoribbons with imperfect edges. We treat different regimes of edge scattering, ranging from wide graphene ribbons with (partially) diffusive edge scattering, to ribbons with large width-variations, and nanoribbons with atomistic edge roughness. For the latter, we consider a pseudopotential approach, allowing for an atomistic treatment of the band structure and the scattering potential, combined with the self-consistent solution of the Boltzmann transport equation within the relaxation-time approximation. The resulting resistivity depends strongly on the ribbon orientation, with zigzag (armchair) ribbons showing the smallest (largest) resistivity, and intermediate ribbon orientations exhibiting intermediate resistivity values. The results also show clear resistivity peaks, corresponding to peaks in the density of states due to the confinement-induced subband quantization, except for armchair-edge ribbons that show a very strong width-dependence because of their 'claromatic' behavior. Furthermore, we identify a strong interplay between the relative position of the two valleys of graphene along the transport direction, the correlation profile of the atomistic edge roughness, and the chiral valley modes, leading to a peculiar strongly suppressed resistivity regime, most pronounced for the zigzag orientation.
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