Shubnikov–de Haas Effect and Angular-Dependent Magnetoresistance in Layered Organic Conductor β′′-(ET)(TCNQ)

This paper reports the experimental results of the Shubnikov–de Haas (SdH) effect and angular-dependent magnetoresistance oscillation (AMRO) for the organic conductor β′′-(ET)(TCNQ). We observed several two dimensional (2D) SdH frequencies, whose cross-sectional areas of the Fermi surfaces (FSs) correspond to only a few percent of the first Brillouin zone. Such small 2D FSs are not predicted by band-structure calculations, suggesting that these FS pockets are created by an imperfect nesting of FSs at low temperatures. It is found that the AMRO consists of a long-period oscillation and a short-period one. The long-period oscillation is associated with the Yamaji oscillation corresponding to the α orbit, whose shape and area are consistent with previous magneto-optical measurement. The short-period oscillation is not caused by peaks instead but dips. The dip structure is discussed in terms of the AMRO of a quasi-2D electron system with a periodic potential caused by the possible density-wave related to the ...