Structure of neutron-rich nuclei and neutron multiplicities in spontaneous fission

Abstract New insights into the fission process and the structure of neutron-rich nuclei have been gained by measuring γ-γ and γ-γ-γ coincidences of the prompt γ-rays following the spontaneous fission of 252 Cf. The data were taken with the Compton Suppression Spectrometer System at HHIRF. New high spin levels were observed in 143,145,147 Ba Only in 143 Ba are intertwined bands observed with the characteristics of the octupole structure found only in 144 Ba. New high spin states observed in the N = 84 136 Te, 138 Xe, 140 Ba nuclei exhibit a symmetry pattern suggestive of a pseudospin f - shell . For the first time in fission, the relative yields and neutron multiplicities were measured directly. Yields and multiplicities were measured directly for the ZrCe and MoBa correlated fragment pairs by observing the coincidences between the γ-rays in each fragment. Zero-neutron to ten-neutron emission yields were determined; the latter for the first time. The zero-neutron emission can be understood as a new example of cluster radioactivity. These results demonstrate that the use of the high resolution γ-γ-γ coincidence technique employed here for the first time opens up a new approach to the study of the fission process that will provide previously inaccessible details of the process.