Surface rippling on bulk metallic glass under nanosecond pulse laser ablation

We report an interesting surface ripple patterns in the irradiated area of a Zr-based bulk metallic glass by nanosecond pulse laser with single shot. Such surface rippling phenomenon can be ascribed to the Kelvin-Helmholtz instability at the interface between the molten layer and the expanding plasma plume. The analytical instability criterion is obtained via a perturbation analysis. Furthermore, the model demonstrates that the characteristic spacing of the ripples is dominated by the density, transverse velocity of the plasma wind, and the surface tension of the molten layer. The predicted spacing agrees well with the experimentally observed values. The results are fundamentally useful for laser-processing bulk metallic glasses (BMGs) and even for understanding the nature of flow in BMGs.