Strong dependence of magnon diffusion in Y3Fe5O12 on light excitation

Tuning the transport behavior of magnons may lead to an energy-efficient technology for information transmission and processing. This stimulates intensive investigations on Y3Fe5O12 (YIG) that exhibits the longest magnon diffusion distance among magnetic materials. While most of the previous works focused on the determination of magnon diffusion length by various techniques, herein we demonstrated how to tune magnon diffusion by laser excitation. We found that the diffusion length is strongly dependent on laser wavelength when the magnon is generated by exposing YIG directly to laser beam. The diffusion length, determined by a nonlocal geometry at room temperature, is ~30 um for the magnons produced by visible light (400-650 nm), and ~160-180 um for the laser between 808 nm and 980 nm. The diffusion distance is much longer than the reported value. In addition to thermal gradient, we found that light illumination affected the electron configuration of the Fe3+ ion in YIG. Long wavelength laser triggers a high spin to low spin state transition of the Fe3+ ions in FeO6 octahedra. This in turn causes a substantial softening of the magnon thus a dramatic increase in diffusion distance. The present work paves the way towards an efficient tuning of magnon transport behavior which is crucially important for magnon spintronics.