Effect of NCl(a~1Δ) Self-annihilation on NCl(a~1Δ) Production and Transfer

The effect of NCl(a~1Δ) self-annihilation on NCl(a~1Δ) production and transfer was simulated by using an one-dimensional premixing reaction model.The results show that the most important factor for NCl(a~1Δ) production and transfer is NCl(a~1Δ) self-annihilation.Although NCl(a~1Δ) self-annihilation effect on NCl(a~1Δ) production and transfer simulated with the data of 2002 is much smaller than that obtained with the data of 1997,the NCl(a~1Δ) self-annihilation is still the most important channel for NCl(a~1Δ) production and transfer losses.The results suggest that it is necessary to do some more work on the measurement of the rate constant of NCl(a~1Δ) self-annihilation reaction and itss dependency on temperature in order to improve the efficiency of NCl(a~1Δ) production and transfer and to analyze and value all-gas-phase laser(AGIL) accurately.