Time evolution of synchronously pumped dye laser pulses: Picosecond pulse formation studies

Abstract The pulse-by-pulse evolution and compression of the output of a synchronously pumped dye laser as a function of the number of pump pulses was investigated with a high resolution, variably triggered streak camera. The measured pulse durations and energies for the pulse compression process are demonstrated to be in disagreement with the predictions of recent classical rate equation models. This is shown not to be due to the complete breakdown of the model but, rather, is caused by the failure to include two key loss terms in the rate equation treatment, namely, excited state absorption and thermal lensing. In addition, a highly durable dye laser compatible with the 100 MHz output of commercially available QS and ML YAG lasers is presented which is capable of 50 μJ, 20–30 ps transform limited pulses without the need of amplification. Further refinements of this laser system are discussed, based on the experimental work reported, which will lead to tunable ∼ 100 fs pulses with energies in the μJ range from a single laser pump source.