Gapless quantum excitations from an icelike splayed ferromagnetic ground state in stoichiometric Yb2Ti2O7

2016 
We know the ground state of the quantum spin ice candidate magnet Yb2Ti2O7 to be sensitive to weak disorder at the similar to 1% level which occurs in single crystals grown from the melt. Powders produced by solid state synthesis tend to be stoichiometric and display large and sharp heat capacity anomalies at relatively high temperatures, T-C similar to 0.26 K. We have carried out neutron elastic and inelastic measurements on well characterized and equilibrated stoichiometric powder samples of Yb2Ti2O7 which show resolution-limited Bragg peaks to appear at low temperatures, but whose onset correlates with temperatures much higher than T-C. The corresponding magnetic structure is best described as an icelike splayed ferromagnet. In the spin dynamics of Yb2Ti2O7 we see the gapless on an energy scale <0.09 meV at all temperatures and organized into a continuum of scattering with vestiges of highly overdamped ferromagnetic spin waves present. These excitations differ greatly from conventional spin waves predicted for Yb2Ti2O7's mean field ordered state, but appear robust to weak disorder as they are largely consistent with those displayed by nonstoichiometric crushed single crystals and single crystals, as well as by powder samples of Yb2Ti2O7's sister quantum magnet Yb2Ti2O7.
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