Unconventional magnetic field response of the hyperhoneycomb Kitaev magnet β−Li2IrO3

We present a unified description of the response of the hyperhoneycomb Kitaev magnet β-Li2IrO3 to appliedmagnetic fields along the orthorhombic directions a, b, and c. This description is based on the minimal nearest-neighbor J-K- model and builds on the idea that the incommensurate counter-rotating order observed experimentally at zero field can be treated as a long-distance twisting of a nearby commensurate order with sixspin sublattices. The results reveal that the behavior of the system for Ha, Hb, and Hc share a number of qualitative features, including (i) a strong intertwining of the modulated, counter-rotating order with a set of uniform orders; (ii) the disappearance of the modulated order at a critical field H∗, whose value is stronglyanisotropic with H∗b ≤H∗a ; (iii) the presence of a robust zigzag phase above H∗; and (iv) the fulfillment of the Bragg peak intensity sum rule. It is noteworthy that the disappearance of the modulated order for Hc proceeds via a “metamagnetic” first-order transition which does not restore all broken symmetries. This implies the existence of a second finite-T phase transition at higher magnetic fields. We also demonstrate that quantum fluctuations give rise to a significant reduction of the local moments for all directions of the field. The results for the total magnetization for Hb are consistent with available data and confirm a previous assertion that the system is very close to the highly frustrated K- line in parameter space. Our predictions for the magnetic response for fields along a and c await experimental verification.