Retrodictive derivation of the radical-ion-pair master equation and Monte Carlo simulation with single-molecule quantum trajectories
2014
Radical-ion-pair reactions, central in photosynthesis and the avian magnetic compass mechanism, have recently shown to be a paradigm system for applying quantum information science in a biochemical setting. The fundamental quantum master equation describing radical-ion-pair reactions is still under debate. We here use quantum retrodiction to produce a rigorous refinement of the theory put forward in Phys. Rev. E {\bf 83}, 056118 (2011). We also provide a rigorous analysis of the measure of singlet-triplet coherence required for deriving the radical-pair master equation. A Monte-Carlo simulation with single-molecule quantum trajectories supports the self-consistency of our approach.
Keywords:
- Correction
- Source
- Cite
- Save
- Machine Reading By IdeaReader
0
References
15
Citations
NaN
KQI