Wearable Fiber-Based Organic Electrochemical Transistors as a Platform for Highly Sensitive Dopamine Monitoring

Fiber-based organic electrochemical transistors (FECTs) provide a new platform for the realization of an ultrafast and ultrasensitive biosensor, especially for the wearable dopamine (DA)-monitoring device. Here, we presented a fully filament-integrated fabric, it exhibited remarkable mechanical compatibility with the human body, and the minimum sensing unit was an organic electrochemical transistor (OECT) based on PVA-co-PE nanofibers (NFs) and polypyrrole (PPy) nanofiber network. The introduction of NFs notably increased the specific surface area and hydrophilicity of the PA6 filament, resulting in the formation of a large area of intertwined PPy nanofiber network. The electrical performance of PPy nanofiber network-modified fibers improved considerably. For the common FECTs, the typical on/off ratio was up to two orders of magnitude, and the temporal recovery time between on and off states was shortened to 0.34 s. Meanwhile, the device exhibited continuous cycling stability. In addition, the performance...