Fragmentation dynamics of methane induced by femtosecond laser pulses
2016
In this study it has been carried out theoretical simulations of ab-initio molecular dynamics of the C–H photo-dissociation of methane induced by femtosecond laser pulses. Our discussion about the reaction mechanism leading to the formation of the H and \(\hbox {CH}_{3}\) fragments is based on the rectification of the Lorentz force. Such an electric force rectification occurs via a periodical charge transfer between H and \(\hbox {CH}_{3}\) induced by the strong infrared laser pulse.
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