Ultrafast metamagnetic phase transition in an elemental antiferromagnet

We present evidence for an ultrafast optically induced antiferromagnetic-to-ferromagnetic phase transition of Mn in Co/Mn multilayers. We observe the transient ferromagnetic signal at the arrival of the pump pulse at the Mn L$_3$ resonance using x-ray magnetic circular dichroism in reflectivity. The timescale of the effect is comparable to the duration of the excitation and occurs before magnetization in Co is quenched. Theoretical calculations point to the imbalanced population of Mn unoccupied states caused by the Co interface for the emergence of this metamagnetic phase transition.