Decoherence and Revival of Attosecond Charge Migration Driven by Non-adiabatic Dynamics
2021
The attosecond quantum beat of an electronic state superposition was captured in SiH4 using soft-X-Ray attosecond transient-absorption spectroscopy. Its decoher-ence and revival, induced by non-adiabatic vibrational dynamics, were reproduced using MCTDH calculations.
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