π-Extended Thiazole-Containing Polymer Semiconductor for Balanced Charge-Carrier Mobilities.
2021
A low-band gap semiconducting polymer with an acceptor-donor-acceptor architecture is newly designed and synthesized by incorporating a π-extended thiazole-vinylene-thiazole unit. The resulting thiazole-containing diketopyrrolopyrrole copolymer exhibits well-balanced ambipolar characteristics with hole mobility of up to 0.11 cm2 V-1 s-1 and electron mobility of up to 0.30 cm2 V-1 s-1 , which are suitable for applications in polymer electronics.
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