Direct Observation of Magnetoelastic Excitations in a Quasi-1D Spiral Magnet

We present a systematic study of spin and lattice dynamics in the quasi-one-dimensional spiral magnet CuBr$_2$, using Raman scattering in conjunction with infrared and neutron spectroscopy as well as first-principles calculation. A rich set of broad Raman bands are observed as spin correlations develop upon cooling. The band energies approximately correspond to sharp optical phonons seen from our Raman and infrared data, and inelastic neutron scattering further reveals that most, if not all, of them are precisely equal to phonon-dispersion energies at the one-dimensional magnetic wave vector. The low-energy bands further exhibit a distinct intensity maximum at the magnetic ordering temperature. Our results point towards the emergence of resonating spin-orbital-lattice textures, or "magnetophonons", at dispersion intersecting points of phonons and spin excitations.