Extreme magnetoresistance and Shubnikov-de Haas oscillations in ferromagnetic DySb.
2018
Rare earth monopnictides represent a novel electronic system for the extremely large magnetoresistance (XMR) and the potential to realize magnetic topological semimetal state, both of which are essential functionalities of electronic materials. In this material family, DySb is a special member, as it undergoes a tetragonal structural transition when it enters antiferromagnetic ground state. Such a ground state can be changed into a ferromagnetic state by magnetic field, via an intermediate phase. In the present paper, we study the electronic structures of DySb under high magnetic field (i.e., in the ferromagnetic state) from both experimental and theoretical aspects. A non-saturated XMR is observed (as large as 3.7*10^4% at 1.8 K and 38.7 T), along with Shubnikov-de Haas (SdH) oscillations. The SdH frequencies are well reproduced by our first principles calculations. Although a band inversion is found theoretically, suggesting that DySb is topologically nontrivial, it is deeply underneath the Fermi level, which rules out a topological nature of the XMR. The XMR is eventually attributed to the compensation mechanism, as evidenced by the nearly equal total densities of electron-like and hole-like carriers, and the high mobility that is associated with the linearly dispersive band at zone corner. This discovery is important to the intensive studies on the XMR of rare earth monopnictides.
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