Coupling Effects of Supercritical CO2 Sequestration in Deep Coal Seam

2019 
CO2 sequestration in deep unminable coal seams is currently identified as a research hot spot to reduce CO2 emissions, due to the potential large-scale storage capacity and complicated physical and chemical reactions, especially for supercritical CO2 (scCO2). Hitherto, the interaction mechanisms between scCO2 and coal mass in situ conditions are still unclear. Therefore, the main objective of this study is to fully address the coupling effects of scCO2 sequestration on coal mass and provide a comprehensive evaluation of the interrelation of these variations. Five cycles of helium and scCO2 injection were replicated on a subbituminous coal sample to investigate the permeability variation with scCO2 saturation time. Meanwhile, gas chromatography–mass spectrometry (GC–MS), gas chromatography (GC), Fourier transform infrared spectroscopy (FTIR), proximate analysis, and low-pressure–temperature nitrogen (N2) isotherm analyses were employed to characterize the transformation in coal mass. The test result shows ...
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