Ground-state order and spin-lattice coupling in tetrahedral spin systems Cu 2 Te 2 O 5 X 2 ( X = Br or Cl)
2004
High-resolution ac susceptibility and thermal conductivity measurement on ${\mathrm{Cu}}_{2}{\mathrm{Te}}_{2}{\mathrm{O}}_{5}{X}_{2}(X=\mathrm{Br},\mathrm{Cl})$ single crystals are reported. For Br-sample, sample dependence prevents one from distinguishing between possibilities of magnetically ordered and spin-singlet ground states. In Cl-sample a three-dimensional transition at 18.5 K is accompanied by almost isotropic behavior of susceptibility and almost switching behavior of thermal conductivity. Thermal conductivity studies suggest the presence of a tremendous spin-lattice coupling characterizing Cl- but not Br-sample. Below the transition Cl-sample is in a complex magnetic state involving AF order but also the elements consistent with the presence of a gap in the excitation spectrum.
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