A general and mild Cu-catalytic N-arylation of iminodibenzyls and iminostilbenes using unactivated aryl halides
2017
A ligand-free, highly efficient Cu-catalytic N-arylation of iminodibenzyl and iminostilbene derivatives with a broad scope of unactivated aryl halides under mild conditions has been developed for the first time. Moreover, the first Ni-based catalytic system was also applied to the N-arylation of pre-existing derivatives. These novel protocols provide facile and convenient access to the construction of dibenzazepines and offer promising alternatives to the widely used palladium catalysts.
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