α‐Hydroxymethylation of Pyridines at a Frustrated Lewis Pair Template
2015
The “η2-formylborane” moiety formed by CO reduction with HB(C6F5)2 at a P/B frustrated Lewis pair template undergoes a hydroxymethylation reaction at the α-position to nitrogen in pyridine or isoquinoline. The analogous reaction with pyrimidine revealed a mechanism related to the Tschitschibabin reaction.
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