Nonequilibrium system-bath entanglement theorem versus heat transport.
2021
In this work, we extend the recently established system{bath entanglement theorem (SBET) [J. Chem. Phys. 152, 034102 (2020)] to the nonequilibrium scenario, in which an arbitrary system couples to multiple Gaussian baths environments at different temperatures. While the existing SBET connects the entangled system{bath response functions to those of local systems, the extended theory is concerned with the nonequilibrium steady{state quantum transport current through molecular junctions. The new theory is established on the basis of the generalized Langevin equation, with a close relation to nonequilibrium thermodynamics in the quantum regime.
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