Cyclic α-Amino Acids via Enantioselective Metal-Catalyzed Cascade Reactions of Dienamides in Supercritical Carbon Dioxide
2005
Highly enantioselective conversion of dienamides into cyclic α-amino acids can be achieved by a single-pot, tandem hydrogenation–hydroformylation–cyclization–elimination sequence using a single catalyst and supercritical carbon dioxide (scCO2) as the reaction solvent at total pressures significantly lower than those previously reported for related hydrogenation and hydroformylation reactions.
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