Ultra Low-level Gamma Ray Spectrometry of Thorium in Human Bone Samples

Following the use of in vivo measurements of 210 Pb to estimate retrospectively radon exposure, interest has been expressed in the use of in vivo measurements of 208 Tl to estimate thorium intake. To aid with calibration and to determine the optimum part of the body on which in vivo measurements should be made, the distribution of 208 Tl and 228 Ac amongst different human bones was measured in the underground laboratory HADES. The 208 Tl activity was determined by the 2614.5 keV and the 583.2 keV gamma ray lines. The 228 Ac activity was determined by the 911.2 keV and the 969.0 keV gamma ray lines. The background under those peaks when measured on the 106% relative efficiency coaxial HPGe detector in HADES is of the order of 1 d -1 , resulting in detection limits in the order of 1 mBq for both radionuclides for a typical 10 g bone sample and for a measuring time of I week.