Te(II)/Te(III) catalyzed cross dehydrogenative C─N bond formation
2020
The Te(II)/Te(III) catalyzed dehydrogenative C─H phenothiazination of challenging phenols featuring electron withdrawing substituents is herein described, under mild aerobic conditions and with high yields. These unexpected Te(II)/Te(III) radical catalytic properties were characterized by cyclic voltammetry, EPR spectroscopy, kinetic experiments and DFT calculations.
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