Solar radiative forcing of aerosol particles near the Taklimakan desert during the Dust Aerosol Observation-Kashi campaign in Spring 2019

Abstract. The Taklimakan desert is a main and continuous source of Asian dust particles causing a significant direct aerosol solar radiative forcing (ASRF). In order to improve the accuracy of the estimation of dust radiative forcing effects, the Dust Aerosol Observation-Kashi (DAO-K) campaign was carried out near the Taklimakan desert in April 2019. The objective of the campaign is to provide comprehensive parameters such as: dust optical and microphysical properties, vertical distribution and surface albedo, for the calculation of ASRF. The measurements were employed in radiative transfer (RT) simulations and the estimations are improved by considering the actual measured atmospheric profiles and diurnal variations of land surface albedo in addition to reliable aerosol parameters. The RT model estimates the ASRF results in average daily mean cooling effects of −19 W m−2 at the top of atmosphere and −36 W m−2 at the bottom of atmosphere during the DAO-K campaign. The Weather Research and Forecasting model with Chemistry (WRF-Chem) with assimilations of the aerosol optical depth and PM2.5 and PM10 concentrations measurements is prone to overestimate the radiative forcing effects of dust aerosols. The percent difference of daily mean ASRF between the two simulations are greater than 50 % in heavy dust episode. Ground-based observations of downward irradiances have validated that the RT simulations are in good agreement with simultaneous observations, whereas the WRF-Chem estimations exhibit obvious discrepancy with these independent measurements. Data assimilations can partly reduce the discrepancy, but there is still room for improving the WRF-Chem simulation of dust aerosol radiative forcing.