Rh(III)-Catalyzed Intramolecular Redox-Neutral Cyclization of Alkenes via C—H Activation
2014
Biologically interesting fused oligocyclic lactams have been prepared via an intramolecular redox-neutral cyclization process. By the proper choice of the substrates with a wide variety of tethered olefins, the less favored C–H bond can be activated and functionalized. This C–H activation proceeds under mild conditions, obviates the need for external oxidants, and displays a broad scope with respect to the substituents.
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