Incineration of 241Am induced by thermal neutrons

Abstract An experimental study of the 241 Am incineration in a high-intensity thermal neutron flux was carried out at the high-flux reactor of the Institut Laue-Langevin in Grenoble. The combination of nuclear γ -ray spectroscopy and off-line mass spectrometry methods made possible the measurement of several parameters of the transmutation chain and the first experimental determination of the unknown 242gs Am thermal neutron capture cross section, which plays an essential role in the 241 Am incineration process. During a 19 days irradiation in a thermal neutron flux of 5.6×10 14 n /( s cm 2 ) , (46±5) % of the initial 241 Am was transmuted by neutron capture of which (22±8) % was incinerated by nuclear fission. A value of the thermal neutron cross section of 242gs Am( n ,γ ) of (330±50) barns was obtained. We show that this keeps the option open to incinerate 241 Am by high-intensity moderated neutron fluxes.