Improving Stability of Cesium Lead Iodide PerovskiteNanocrystals by Solution Surface Treatments
2020
Cesium
lead halide perovskite nanocrystals have a narrow emission
peak tunable in the visible wavelength range with a high quantum yield.
They hold great potential for optoelectronic applications such as
light-emitting diodes or electronic displays. However, cesium lead
iodide (CsPbI3) is not stable under ambient conditions,
limiting its applications. Here, we use a solution surface treatment
approach to improve the photostability of CsPbI3 suspensions
in toluene. When a CsPbBr3 precursor is used via the method
of heterogeneous surface treatment, the photoluminescence (PL) intensity
is enhanced but the PL only lasts 2 days. In contrast, when a CsPbI3 precursor is used via the method of homogeneous surface treatment,
not only the PL intensity of CsPbI3 suspensions is enhanced
but also the stability with the PL lasts for 11 days. It is likely
that a better protection on the core CsPbI3 by itself can
be achieved because of better matching of the material structure and
surface chemistry.
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